Some others that you may have interest in...
TV series:
If you liked Samurai Champloo, I'd suggest "Cowboy Beebop" and/or "Trigun". Fullmetal Alchemist carried on the series with "Brotherhood". If you liked Blood+, then I suggest "Witchblade, the animated series". And for Big O, I suggest "Escaflowne" or the "Gundam" series (Never did like the oversized robots series). And if you want a good fantasy series, then I suggest "The Twelve Kingdoms".
Attack on Titan...I love the way they animate those giants. You may want to try out "Beezlebub" and/or "Baki the Grappler"...a little crazy, but you may like these as well.
Of course, I have to mention Dragonball and Dragonball Z! Pass on the GT series though...
Movies:
If you like Spirited Away and Kiki's Delivery Service, then I suggest any of Studio Glibli's films, but I'd start off with "Princess Mononoke", then "Howl's Moving Castle", and on to all the others that are available...they're all amazing.
One that I don't see on here, which I thought was really good, was "Summer Wars".
I'm sure you can find most, if not all, on Crunchyroll. Hope you enjoy!
Shout by raya (mango)BlockedParent2013-11-05T00:13:32Z
Someone I know recently finished Cowboy Bebop and recommended it to me. It looks great from what I have seen, and it's right near the top on my to-watch list! I should watch it after I finish Brotherhood.
Thanks for the recommendations, I'll look into them!